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A few years ago, our group started to systematically analyse this class of organic electron-donor compounds. 6, 7 Compounds 1–3 (see Figure 1) were synthesised and their redox potentials determined. 8 Compounds 1 and 2 were used as ligands in zinc(II), 9 cobalt(II) 8 and copper(II) 10 complexes, featuring a rather …
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Two homoleptic copper(II) complexes [Cu(L1) 2] and [Cu(L2) 2] with anionic redox-active ligands were synthesised, one with urea azine (L1) and the other with thio-urea azine (L2) ligands.One-electron oxidation of the complexes initiates an unprecedented redox-induced electron transfer process, leading to monocationic copper(I) complexes …
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